A New Spin on Atoms Gives Scientists a Closer Look at Quantum Weirdness

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A research team has developed a new way to control and measure atoms that are so close together no optical lens can distinguish them. Artist’s rendering by Rachel Davidowitz

A team of Princeton researchers have developed a new way to control and measure atoms that are so close together no optical lens can distinguish them, according to Princeton news.

Described in an article published Oct. 30 in the journal Science, their method excites closely-spaced erbium atoms in a crystal using a finely tuned laser in a nanometer-scale optical circuit.  The researchers, led by Jeff Thompson, an assistant professor of Electrical Engineering, take advantage of the fact that each atom responds to slightly different frequencies, or colors, of laser light, allowing the researchers to resolve and control multiple atoms, without relying on their spatial information.

In a conventional microscope, the space between two atoms effectively disappears when their separation is below a key distance called the diffraction limit, which is roughly equal to the light’s wavelength. This is analogous to two distant stars that appear as a single point of light in the night sky. However, this is also the scale at which atoms start to interact and give rise to rich and interesting quantum mechanical behavior.

“We always wonder, at the most fundamental level — inside solids, inside crystals — what do atoms actually do? How do they interact?” said physicist Andrei Faraon, a professor at the California Institute of Technology who was not involved in the research. “This [paper] opens the window to study atoms that are in very, very close proximity.”

Introducing TQI 2.0Introducing TQI 2.0

Studying atoms and their interactions at tiny distances allows scientists to explore and control a quantum property known as spin.

Studying atoms and their interactions at tiny distances allows scientists to explore and control a quantum property known as spin. As a form of momentum, spin is usually described as being either up or down (or both, but that’s another story). When the distance between two atoms grows vanishingly small — mere billionths of a meter — the spin of one exerts influence over the spin of the other, and vice versa. As spins interact in this realm, they can become entangled, a term scientists use to describe two or more particles that are inextricably linked. Entangled particles behave as if they share one existence, no matter how far apart they later become. Entanglement is the essential phenomenon that separates quantum mechanics from the classical world, and it’s at the center of the vision for quantum technologies. The new Princeton device is a stepping stone for scientists to study these spin interactions with unprecedented clarity.

One important feature of the new Princeton device is its potential to address hundreds of atoms at a time, providing a rich quantum laboratory in which to gather empirical data. It’s a boon for physicists who hope to unlock reality’s deepest mysteries, including the spooky nature of entanglement.

Such inquiry is not merely esoteric. Over the past three decades, engineers have sought to use quantum phenomena to create complex technologies for information processing and communication, from the logical building blocks of emerging quantum computers, capable of solving otherwise impossible problems, to ultrasecure communication methods that can link machines into an unhackable quantum Internet. To develop these systems further, scientists will need to entangle particles reliably and exploit their entanglement to encode and process information.

Thompson’s team saw an opportunity in erbium. Traditionally used in lasers and magnets, erbium was not widely explored for use in quantum systems because it is difficult to observe, according to the researchers. The team made a breakthrough in 2018, developing a way to enhance the light emitted by these atoms, and to detect that signal extremely efficiently. Now they’ve shown they can do it all en masse.

When the laser illuminates the atoms, it excites them just enough for them to emit a faint light at a unique frequency, but delicately enough to preserve and read out the atoms’ spins. These frequencies change ever so subtly according to the atoms’ different states, so that “up” has one frequency and “down” has another, and each individual atom has its own pair of frequencies.

“If you have an ensemble of these qubits, they all emit light at very slightly different frequencies. And so by tuning the laser carefully to the frequency of one or the frequency of the other, we can address them, even though we have no ability to spatially resolve them,” Thompson said. “Each atom sees all of the light, but they only listen to the frequency they’re tuned to.”

The light’s frequency is then a perfect proxy for the spin. Switching the spins up and down gives researchers a way to make calculations. It’s akin to transistors that are either on or off in a classical computer, giving rise to the zeroes and ones of our digital world.

“We want to make them close so we can have this mutual interaction, and use this interaction to create a quantum logic gate.”

To form the basis of a useful quantum processor, these qubits will need to go a step further.

“The strength of the interaction is related to the distance between the two spins,” said Songtao Chen, a postdoctoral researcher in Thompson’s lab and one of the paper’s two lead authors. “We want to make them close so we can have this mutual interaction, and use this interaction to create a quantum logic gate.”

A quantum logic gate requires two or more entangled qubits, making it capable of performing uniquely quantum operations, such as computing the folding patterns of proteins or routing information on the quantum internet.

Thompson, who holds a leadership position at the U.S. Department of Energy‘s new $115M quantum science initiative(link is external), is on a mission to bring these qubits to heel. Within the materials area of the Co-Design Center for Quantum Advantage, he leads the sections on qubits for computing and networking.

His erbium system, a new kind of qubit that is especially useful in networking applications, can operate using the existing telecommunications infrastructure, sending signals in the form of encoded light over silicon devices and optical fibers. These two properties give erbium an industrial edge over today’s most advanced solid-state qubits, which transmit information through visible light wavelengths that don’t work well with optical-fiber communication networks.

Still, to operate at scale, the erbium system will need to be further engineered.

While the team can control and measure the spin state of its qubits no matter how close they get, and use optical structures to produce high-fidelity measurement, they can’t yet arrange the qubits as needed to form two-qubit gates. To do that, engineers will need to find a different material to host the erbium atoms. The study was designed with this future improvement in mind.

“One of the major advantages of the way we have done this experiment is that it has nothing to do with what host the erbium sits in,” said Mouktik Raha, a sixth-year graduate student in electrical engineering and one of the paper’s two lead authors. “As long as you can put erbium inside it and it doesn’t jitter around, you’re good to go.”

Christopher M. Phenicie and Salim Ourari, both electrical engineering graduate students, also contributed to the paper. The work was carried out in conjunction with the Princeton Quantum Initiative(link is external), and funded in part by the National Science Foundation, the Princeton Center for Complex Materials, the Young Investigator Program of the Air Force Office of Scientific Research, and the Defense Advanced Research Projects Agency.

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Princeton University
UniversityUnited States · 5001-10000 FTEs

Princeton University is a private Ivy League research institution located in Princeton, New Jersey. It traces its roots back to 1746 when it was established as the College of New Jersey in Elizabeth. Being one of the United States' oldest higher education institutions, it's now recognized as the fourth-oldest. The university transitioned through various locations, finally settling in its current site. It achieved university status in 1896 and was later renamed Princeton University.

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California Institute of Technology
UniversityUnited States · 1001-5000 FTEs

The California Institute of Technology, situated in Pasadena, California, is a private research university. It has played a crucial role in numerous contemporary scientific breakthroughs and stands alongside a select few technology institutes in the United States that prioritize teaching in pure and applied sciences.

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U.S. Department of Energy (DOE)
GovernmentUnited States · 10001+ FTEs

The mission of the Department of Energy is to ensure America's security and prosperity by addressing its energy, environmental, and nuclear challenges through transformative science and technology solutions. In September, 2022, Research supported by ASCR demonstrated that classical machine learning algorithms can accurately predict ground state properties and classify quantum phases of matter using data generated from quantum experiments. In November, 2022, Research supported by Q-NEXT revealed that the performance of a sensor network is constrained by the intrinsic noise associated with the quantum states used in the network. In March, 2023, Research funded by DOE SC NP achieved the first experimental observation of entanglement between dissimilar particles, specifically positive and negative pions. In August, 2023, Research funded by DOE SC BER demonstrated strong preservation of entanglement in a two-photon absorption process involving organic molecules, offering a new approach for developing quantum light-based spectroscopy and microscopy.

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Defense Advanced Research Projects Agency (DARPA)
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The Defense Advanced Research Projects Agency (DARPA) is an independent research and development agency within the U.S. Department of Defense (DoD) established in 1958 to prevent and create strategic technological surprises for national security. Operating with a relatively small staff of program managers who are empowered to take high-risk, high-reward approaches, DARPA functions by funding cutting-edge research in academia, industry, and government laboratories rather than conducting research in-house. Its mission focuses on creating revolutionary technologies—such as the Internet (ARPANET), stealth technology, GPS, and mRNA vaccine platforms—that transition into practical military and civilian applications. DARPA programs are typically finite in duration and demand transformational breakthroughs rather than incremental improvements, positioning the U.S. at the forefront of technological innovation.

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